Diketopyrrolopyrrole-based Conjugated Polymers as Representative Semiconductors for High-Performance Organic Thin-Film Transistors and Circuits

Kai-Qing Liu; Yuan-He Gu; Zheng-Ran Yi; Yun-Qi Liu

doi:10.1007/s10118-023-2943-1

Your Location：

Home >

Browse articles >

Diketopyrrolopyrrole-based Conjugated Polymers as Representative Semiconductors for High-Performance Organic Thin-Film Transistors and Circuits

REVIEW | Updated：2023-04-21

- Diketopyrrolopyrrole-based Conjugated Polymers as Representative Semiconductors for High-Performance Organic Thin-Film Transistors and Circuits
- Chinese Journal of Polymer Science Vol. 41, Issue 5, Pages: 671-682(2023)
- Affiliations：
  
  a.Zhuhai Fudan Innovation Institution, Zhuhai 518057, China
  b.Department of Environmental Science and Engineering, Faculty of Innovation Engineering, Macau University of Science and Technology, Macau 999078, China
  c.Key Laboratory of Organic Solids, Beijing National Laboratory for Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China
- Author bio：
  
  yzr@whu.edu.cn(Z.R.Y.)
  liuyq@iccas.ac.cn(Y.Q.L.)
- Funds：
- DOI：10.1007/s10118-023-2943-1
  CLC：
- Received：04 December 2022，
  
  Revised：2022-12-25，
  
  Accepted：31 December 2022，
  
  Online First：03 March 2023，
  
  Published：01 May 2023
- Accepted：
Scan QR Code
Liu, K. Q.; Gu, Y. H.; Yi, Z. R.; Liu, Y. Q. Diketopyrrolopyrrole-based conjugated polymers as representative semiconductors for high-performance organic thin-film transistors and circuits.Chinese J. Polym. Sci.2023,41, 671–682

Kai-Qing Liu, Yuan-He Gu, Zheng-Ran Yi, et al. Diketopyrrolopyrrole-based Conjugated Polymers as Representative Semiconductors for High-Performance Organic Thin-Film Transistors and Circuits[J]. Chinese Journal of Polymer Science, 2023, 41(5): 671-682.
Liu, K. Q.; Gu, Y. H.; Yi, Z. R.; Liu, Y. Q. Diketopyrrolopyrrole-based conjugated polymers as representative semiconductors for high-performance organic thin-film transistors and circuits.Chinese J. Polym. Sci.2023,41, 671–682 DOI： 10.1007/s10118-023-2943-1.

Kai-Qing Liu, Yuan-He Gu, Zheng-Ran Yi, et al. Diketopyrrolopyrrole-based Conjugated Polymers as Representative Semiconductors for High-Performance Organic Thin-Film Transistors and Circuits[J]. Chinese Journal of Polymer Science, 2023, 41(5): 671-682. DOI： 10.1007/s10118-023-2943-1.

摘要

The review summarizes the progress in molecular design

synthesis and solution-processing of DPP-based conjugated polymers for OTFT devices and circuits. The important roles of design strategies

synthesis methods and processing techniques are highlighted and discussed.

Abstract

Since the first report of diketopyrrolopyrrole (DPP)-based conjugated polymers for organic thin-film transistors (OTFTs)

these polymers have attracted great attention as representative semiconductors in high-performance OTFTs. Through unremitting efforts in molecular-structure regulation and device optimization

significant mobilities exceeding 10 cm

·V

–1

·s

–1

have been achieved in OTFTs

greatly promoting the applied development of organic circuits. In this review

we summarize our progress in molecular design

synthesis and solution-processing of DPP-based conjugated polymers for OTFT devices and circuits

focusing on the roles of design strategies

synthesis methods and processing techniques. Furthermore

the remaining issues and future outlook in the field are briefly discussed.

关键词

Keywords

references

Wu, Y.; Zhao, Y.; Liu, Y . Toward efficient charge transport of polymer-based organic field-effect transistors: molecular design, processing, and functional utilization . Acc. Mater. Res. , 2021 , 2 1047 - 1058 . DOI: 10.1021/accountsmr.1c00149 http://doi.org/10.1021/accountsmr.1c00149 .

Yang, J.; Zhao, Z.; Wang, S.; Guo, Y.; Liu, Y . Insight into high-performance conjugated polymers for organic field-effect transistors . Chem , 2018 , 4 2748 - 2785 . DOI: 10.1016/j.chempr.2018.08.005 http://doi.org/10.1016/j.chempr.2018.08.005 .

Yan, Y.; Zhao, Y.; Liu, Y . Recent progress in organic field-effect transistor-based integrated circuits . J. Polym. Sci. , 2022 , 60 311 - 327 . DOI: 10.1002/pol.20210457 http://doi.org/10.1002/pol.20210457 .

Pei, K.; Chen, M.; Zhou, Z.; Li, H.; Chan, P. K. L . Overestimation of carrier mobility in organic thin film transistors due to unaccounted fringe currents . ACS Appl. Electron. Mater. , 2019 , 1 379 - 388 . DOI: 10.1021/acsaelm.8b00097 http://doi.org/10.1021/acsaelm.8b00097 .

Snyder, G. J.; Snyder, A. H.; Wood, M.; Gurunathan, R.; Snyder, B. H.; Niu, C . Weighted mobility . Adv. Mater. , 2020 , 32 2001537 DOI: 10.1002/adma.202001537 http://doi.org/10.1002/adma.202001537 .

Fratini, S.; Ciuchi, S.; Mayou, D.; de Laissardière, G. T.; Troisi, A . A map of high-mobility molecular semiconductors . Nat. Mater. , 2017 , 16 998 - 1002 . DOI: 10.1038/nmat4970 http://doi.org/10.1038/nmat4970 .

Takimiya, K.; Shinamura, S.; Osaka, I.; Miyazaki, E . Thienoacene-based organic semiconductors . Adv. Mater. , 2011 , 23 4347 - 4370 . DOI: 10.1002/adma.201102007 http://doi.org/10.1002/adma.201102007 .

Zhang, Z.; Peng, B.; Ji, X.; Pei, K.; Chan, P. K. L . Marangoni-effect-assisted bar-coating method for high-quality organic crystals with compressive and tensile strains . Adv. Funct. Mater. , 2017 , 27 1703443 DOI: 10.1002/adfm.201703443 http://doi.org/10.1002/adfm.201703443 .

Wang, Y.; Hasegawa, T.; Matsumoto, H.; Michinobu, T . Significant improvement of unipolar N-type transistor performances by manipulating the coplanar backbone conformation of electron-deficient polymers via hydrogen bonding . J. Am. Chem. Soc. , 2019 , 141 3566 - 3575 . DOI: 10.1021/jacs.8b12499 http://doi.org/10.1021/jacs.8b12499 .

Wadsworth, A.; Chen, H.; Thorley, K. J.; Cendra, C.; Nikolka, M.; Bristow, H.; Moser, M.; Salleo, A.; Anthopoulos, T. D.; Sirringhaus, H.; McCulloch, I . Modification of indacenodithiophene-based polymers and its impact on charge carrier mobility in organic thin-film transistors . J. Am. Chem. Soc. , 2020 , 142 652 - 664 . DOI: 10.1021/jacs.9b09374 http://doi.org/10.1021/jacs.9b09374 .

Gao, Y.; Deng, Y.; Tian, H.; Zhang, J.; Yan, D.; Geng, Y.; Wang, F . Multifluorination toward high-mobility ambipolar and unipolar n-type donor-acceptor conjugated polymers based on isoindigo . Adv. Mater. , 2017 , 29 1606217 DOI: 10.1002/adma.201606217 http://doi.org/10.1002/adma.201606217 .

Xu, L.; Zhao, Z.; Xiao, M.; Yang, J.; Xiao, J.; Yi, Z.; Wang, S.; Liu, Y. . π -Extended isoindigo-based derivative: a promising electron-deficient building block for polymer semiconductors . ACS Appl. Mater. Interfaces , 2017 , 9 40549 - 40555 . DOI: 10.1021/acsami.7b13570 http://doi.org/10.1021/acsami.7b13570 .

Yan, X.; Xiong, M.; Li, J. T.; Zhang, S.; Ahmad, Z.; Lu, Y.; Wang, Z. Y.; Yao, Z. F.; Wang, J. Y.; Gu, X.; Lei, T . Pyrazine-flanked diketopyrrolopyrrole (DPP): a new polymer building block for high-performance n-type organic thermoelectrics . J. Am. Chem. Soc. , 2019 , 141 20215 - 20221 . DOI: 10.1021/jacs.9b10107 http://doi.org/10.1021/jacs.9b10107 .

Yan, X.; Xiong, M.; Deng, X. Y.; Liu, K. K.; Li, J. T.; Wang, X. Q.; Zhang, S.; Prine, N.; Zhang, Z.; Huang, W.; Wang, Y.; Wang, J. Y.; Gu, X.; So, S. K.; Zhu, J.; Lei, T . Approaching disorder-tolerant semiconducting Polymers . Nat. Commun. , 2021 , 12 5723 DOI: 10.1038/s41467-021-26043-y http://doi.org/10.1038/s41467-021-26043-y .

Xiong, M.; Yan, X.; Li, J.-T.; Zhang, S.; Cao, Z.; Prine, N.; Lu, Y.; Wang, J. Y.; Gu, X.; Lei, T . Efficient N-doping of polymeric semiconductors through controlling the dynamics of solution-state polymer aggregates . Angew. Chem. , 2021 , 133 8270 - 8278 . DOI: 10.1002/ange.202015216 http://doi.org/10.1002/ange.202015216 .

Feng, K.; Guo, H.; Sun, H.; Guo, X . N-type organic and polymeric semiconductors based on bithiophene imide derivatives . Acc. Chem. Res. , 2021 , 54 3804 - 3817 . DOI: 10.1021/acs.accounts.1c00381 http://doi.org/10.1021/acs.accounts.1c00381 .

Chen, X. X.; Li, J. T.; Fang, Y. H.; Deng, X. Y.; Wang, X. Q.; Liu, G.; Wang, Y.; Gu, X.; Jiang, S. D.; Lei, T . High-mobility semiconducting polymers with different spin ground states . Nat. Commun. , 2022 , 13 2258 DOI: 10.1038/s41467-022-29918-w http://doi.org/10.1038/s41467-022-29918-w .

Chen, Z.; Lee, M. J.; Shahid Ashraf, R.; Gu, Y.; Albert-Seifried, S.; Meedom Nielsen, M.; Schroeder, B.; Anthopoulos, T. D.; Heeney, M.; McCulloch, I.; Sirringhaus, H . High-performance ambipolar diketopyrrolopyrrole-thieno[3,2- b ]thiophene copolymer field-effect transistors with balanced hole and electron mobilities . Adv. Mater. , 2012 , 24 647 - 652 . DOI: 10.1002/adma.201102786 http://doi.org/10.1002/adma.201102786 .

Lee, J. S.; Son, S. K.; Song, S.; Kim, H.; Lee, D. R.; Kim, K.; Ko, M. J.; Choi, D. H.; Kim, B.; Cho, J. H . Importance of solubilizing group and backbone planarity in low band gap polymers for high performance ambipolar field-effect transistors . Chem. Mater. , 2012 , 24 1316 - 1323 . DOI: 10.1021/cm2037487 http://doi.org/10.1021/cm2037487 .

Yi, Z.; Wang, S.; Liu, Y . Design of high-mobility diketopyrrolopyrrole-based π -conjugated copolymers for organic thin-film transistors . Adv. Mater. , 2015 , 27 3589 - 3606 . DOI: 10.1002/adma.201500401 http://doi.org/10.1002/adma.201500401 .

Ran, Y.; Guo, Y.; Liu, Y . Organostannane-free polycondensation and eco-friendly processing strategy for the design of semiconducting polymers in transistors . Mater. Horiz. , 2020 , 7 1955 - 1970 . DOI: 10.1039/D0MH00138D http://doi.org/10.1039/D0MH00138D .

Li, J.; Zhao, Y.; Tan, H. S.; Guo, Y.; Di, C. A.; Yu, G.; Liu, Y.; Lin, M.; Lim, S. H.; Zhou, Y.; Su, H.; Ong, B. S . A stable solution-processed polymer semiconductor with record high-mobility for printed transistors . Sci. Rep. , 2012 , 2 754 - 763 . DOI: 10.1038/srep00754 http://doi.org/10.1038/srep00754 .

Grozema, F. C.; van Duijnen, P . Th.; Berlin, Y. A.; Ratner, M. A.; Siebbeles, L. D. A. Intramolecular charge transport along isolated chains of conjugated polymers: effect of torsional disorder and polymerization defects . J. Phys. Chem. B , 2002 , 106 7791 - 7795 . DOI: 10.1021/jp021114v http://doi.org/10.1021/jp021114v .

Yi, Z.; Jiang, Y.; Xu, L.; Zhong, C.; Yang, J.; Wang, Q.; Xiao, J.; Liao, X.; Wang, S.; Guo, Y.; Hu, W.; Liu, Y . Triple acceptors in a polymeric architecture for balanced ambipolar transistors and high-gain inverters . Adv. Mater. , 2018 , 30 1801951 DOI: 10.1002/adma.201801951 http://doi.org/10.1002/adma.201801951 .

Sun, B.; Hong, W.; Yan, Z.; Aziz, H.; Li, Y . Record high electron mobility of 6.3 cm 2 V −1 s −1 achieved for polymer semiconductors using a new building block . Adv. Mater. , 2014 , 26 2636 - 2642 . DOI: 10.1002/adma.201305981 http://doi.org/10.1002/adma.201305981 .

Chen, M. S.; Lee, O. P.; Niskala, J. R.; Yiu, A. T.; Tassone, C. J.; Schmidt, K.; Beaujuge, P. M.; Onishi, S. S.; Toney, M. F.; Zettl, A.; Fréchet, J. M. J . Enhanced solid-state order and field-effect hole mobility through control of nanoscale polymer aggregation . J. Am. Chem. Soc. , 2013 , 135 19229 - 19236 . DOI: 10.1021/ja4088665 http://doi.org/10.1021/ja4088665 .

Lei, T.; Dou, J. H.; Cao, X. Y.; Wang, J. Y.; Pei, J . A BDOPV-based donor-acceptor polymer for high-performance n-type and oxygen-doped ambipolar field-effect transistors . Adv. Mater. , 2013 , 25 6589 - 6593 . DOI: 10.1002/adma.201302278 http://doi.org/10.1002/adma.201302278 .

Sirringhaus, H. . 25 th Anniversary article: organic field-effect transistors: the path beyond amorphous silicon . Adv. Mater. , 2014 , 26 1319 - 1335 . DOI: 10.1002/adma.201304346 http://doi.org/10.1002/adma.201304346 .

Guo, X.; Facchetti, A.; Marks, T. J . Imide- and amide-functionalized polymer semiconductors . Chem. Rev. , 2014 , 114 8943 - 9021 . DOI: 10.1021/cr500225d http://doi.org/10.1021/cr500225d .

Sirringhaus, H.; Brown, P. J.; Friend, R. H.; Nielsen, M. M.; Bechgaard, K.; Langeveld-Voss, B. M. W.; Spiering, A. J. H.; Janssen, R. a. J.; Meijer, E. W.; Herwig, P.; de Leeuw, D. M . Two-dimensional charge transport in self-organized, high-mobility conjugated polymers . Nature , 1999 , 401 685 - 688 . DOI: 10.1038/44359 http://doi.org/10.1038/44359 .

McCulloch, I.; Heeney, M.; Bailey, C.; Genevicius, K.; MacDonald, I.; Shkunov, M.; Sparrowe, D.; Tierney, S.; Wagner, R.; Zhang, W.; Chabinyc, M. L.; Kline, R. J.; McGehee, M. D.; Toney, M. F . Liquid-crystalline semiconducting polymers with high charge-carrier mobility . Nat. Mater. , 2006 , 5 328 - 333 . DOI: 10.1038/nmat1612 http://doi.org/10.1038/nmat1612 .

Yi, Z.; Sun, X.; Zhao, Y.; Guo, Y.; Chen, X.; Qin, J.; Yu, G.; Liu, Y . Diketopyrrolopyrrole-based π -conjugated copolymer containing β -unsubstituted quintetthiophene unit: a promising material exhibiting high hole-mobility for organic thin-film transistors . Chem. Mater. , 2012 , 24 4350 - 4356 . DOI: 10.1021/cm302341m http://doi.org/10.1021/cm302341m .

Yi, Z.; Ma, L.; Chen, B.; Chen, D.; Chen, X.; Qin, J.; Zhan, X.; Liu, Y.; Ong, W. J.; Li, J . Effect of the longer β -unsubstituted oliogothiophene unit (6T and 7T) on the organic thin-film transistor performances of diketopyrrolopyrrole-oliogo- thiophene copolymers . Chem. Mater. , 2013 , 25 4290 - 4296 . DOI: 10.1021/cm402381w http://doi.org/10.1021/cm402381w .

Chen, H.; Guo, Y.; Yu, G.; Zhao, Y.; Zhang, J.; Gao, D.; Liu, H.; Liu, Y . Highly π -extended copolymers with diketopyrrolopyrrole moieties for high-performance field-effect transistors . Adv. Mater. , 2012 , 24 4618 - 4622 . DOI: 10.1002/adma.201201318 http://doi.org/10.1002/adma.201201318 .

Pan, H.; Li, Y.; Wu, Y.; Liu, P.; Ong, B. S.; Zhu, S.; Xu, G . Low-temperature, solution-processed, high-mobility polymer semiconductors for thin-film transistors . J. Am. Chem. Soc. , 2007 , 129 4112 - 4113 . DOI: 10.1021/ja067879o http://doi.org/10.1021/ja067879o .

Sonar, P.; Singh, S. P.; Li, Y.; Soh, M. S.; Dodabalapur, A . A low-bandgap diketopyrrolopyrrole-benzothiadiazole-based copolymer for high-mobility ambipolar organic thin-film transistors . Adv. Mater. , 2010 , 22 5409 - 5413 . DOI: 10.1002/adma.201002973 http://doi.org/10.1002/adma.201002973 .

Yamashita, Y . Development of high-performance n-type organic field-effect transistors based on nitrogen heterocycles . Chem. Lett. , 2009 , 38 870 - 875 . DOI: 10.1246/cl.2009.870 http://doi.org/10.1246/cl.2009.870 .

Li, P.; Wang, H.; Ma, L.; Xu, L.; Xiao, F.; Yi, Z.; Liu, Y.; Wang, S . An isoindigo-bithiazole-based acceptor-acceptor copolymer for balanced ambipolar organic thin-film transistors . Sci. China Chem. , 2016 , 59 679 - 683 . DOI: 10.1007/s11426-015-0511-9 http://doi.org/10.1007/s11426-015-0511-9 .

Cheng, C.; Yu, C.; Guo, Y.; Chen, H.; Fang, Y.; Yu, G.; Liu, Y . A diketopyrrolopyrrole–thiazolothiazole copolymer for high performance organic field-effect transistors . Chem. Commun. , 2013 , 49 1998 - 2000 . DOI: 10.1039/c2cc38811a http://doi.org/10.1039/c2cc38811a .

Li, P.; Xu, L.; Shen, H.; Duan, X.; Zhang, J.; Wei, Z.; Yi, Z.; Di, C.; Wang, S . D–A1–D–A2 copolymer based on pyridine-capped diketopyrrolopyrrole with fluorinated benzothiadiazole for high-performance ambipolar organic thin-film transistors . ACS Appl. Mater. Interfaces , 2016 , 8 8620 - 8626 . DOI: 10.1021/acsami.5b12050 http://doi.org/10.1021/acsami.5b12050 .

Yang, J.; Wang, H.; Chen, J.; Huang, J.; Jiang, Y.; Zhang, J.; Shi, L.; Sun, Y.; Wei, Z.; Yu, G.; Guo, Y.; Wang, S.; Liu, Y . Bis-diketopyrrolopyrrole moiety as a promising building block to enable balanced ambipolar polymers for flexible transistors . Adv. Mater. , 2017 , 29 1606162 DOI: 10.1002/adma.201606162 http://doi.org/10.1002/adma.201606162 .

Shen, T.; Li, W.; Zhao, Y.; Liu, Y.; Wang, Y . An all-C–H-activation strategy to rapidly synthesize high-mobility well-balanced ambipolar semiconducting polymers . Matter , 2022 , 5 1953 - 1968 . DOI: 10.1016/j.matt.2022.04.008 http://doi.org/10.1016/j.matt.2022.04.008 .

Babel, A.; Jenekhe, S. A . Alkyl chain length dependence of the field-effect carrier mobility in regioregular poly(3-alkylthiophene)s . Synth. Metals , 2005 , 148 169 - 173 . DOI: 10.1016/j.synthmet.2004.09.033 http://doi.org/10.1016/j.synthmet.2004.09.033 .

Yi, Z.; Ma, L.; Li, P.; Xu, L.; Zhan, X.; Qin, J.; Chen, X.; Liu, Y.; Wang, S . Enhancing the organic thin-film transistor performance of diketopyrrolopyrrole–benzodithiophene copolymers via the modification of both conjugated backbone and side chain . Polym. Chem. , 2015 , 6 5369 - 5375 . DOI: 10.1039/C5PY00704F http://doi.org/10.1039/C5PY00704F .

Zhou, D.; Doumon, Y. N.; Abdu-Aguye, M.; Bartesaghi, D.; Loi, A. M.; Koster, L. J. A.; Chiechi, C. R.; Hummelen, C. J . High-quality conjugated polymers via one-pot Suzuki-Miyaura homopolymerization . RSC Adv. , 2017 , 7 27762 - 27769 . DOI: 10.1039/C7RA03539J http://doi.org/10.1039/C7RA03539J .

Murage, J.; Eddy, J. W.; Zimbalist, J. R.; McIntyre, T. B.; Wagner, Z. R.; Goodson, F. E . Effect of reaction parameters on the molecular weights of polymers formed in a suzuki polycondensation . Macromolecules , 2008 , 41 7330 - 7338 . DOI: 10.1021/ma801275y http://doi.org/10.1021/ma801275y .

Carrillo, J. A.; Turner, M. L.; Ingleson, M. J . A general protocol for the polycondensation of thienyl N -methyliminodiacetic acid boronate esters to form high molecular weight copolymers . J. Am. Chem. Soc. , 2016 , 138 13361 - 13368 . DOI: 10.1021/jacs.6b07666 http://doi.org/10.1021/jacs.6b07666 .

Hoch, M . Organotin compounds in the environment—an overview . Appl. Geochem. , 2001 , 16 719 - 743 . DOI: 10.1016/S0883-2927(00)00067-6 http://doi.org/10.1016/S0883-2927(00)00067-6 .

Wang, Q.; Takita, R.; Kikuzaki, Y.; Ozawa, F . Palladium-catalyzed dehydrohalogenative polycondensation of 2-bromo-3-hexylthiophene: an efficient approach to head-to-tail poly(3-hexylthiophene) . J. Am. Chem. Soc. , 2010 , 132 11420 - 11421 . DOI: 10.1021/ja105767z http://doi.org/10.1021/ja105767z .

Ponder Jr, J. F.; Chen, H.; Luci, A. M. T.; Moro, S.; Turano, M.; Hobson, A. L.; Collier, G. S.; Perdigão, L. M. A.; Moser, M.; Zhang, W.; Costantini, G.; Reynolds, J. R.; McCulloch, I . Low-defect, high molecular weight indacenodithiophene (IDT) polymers via a C–H activation: evaluation of a simpler and greener approach to organic electronic materials . ACS Mater. Lett. , 2021 , 3 1503 - 1512 . DOI: 10.1021/acsmaterialslett.1c00478 http://doi.org/10.1021/acsmaterialslett.1c00478 .

Bura, T.; Beaupré, S.; Légaré, M. A.; Quinn, J.; Rochette, E.; Terence Blaskovits, J.; Fontaine, F. G.; Pron, A.; Li, Y.; Leclerc, M . Direct heteroarylation polymerization: guidelines for defect-free conjugated polymers . Chem. Sci. , 2017 , 8 3913 - 3925 . DOI: 10.1039/C7SC00589J http://doi.org/10.1039/C7SC00589J .

Yi, Z.; Yan, Y.; Wang, H.; Li, W.; Liu, K.; Zhao, Y.; Gu, G.; Liu, Y . Chain-extending polymerization for significant improvement in organic thin-film transistor performance . ACS Appl. Mater. Interfaces , 2022 , 14 36918 - 36926 . DOI: 10.1021/acsami.2c10133 http://doi.org/10.1021/acsami.2c10133 .

Zhang, F.; Di, C.; Berdunov, N.; Hu, Y.; Hu, Y.; Gao, X.; Meng, Q.; Sirringhaus, H.; Zhu, D . Ultrathin film organic transistors: precise control of semiconductor thickness via spin-coating . Adv. Mater. , 2013 , 25 1401 - 1407 . DOI: 10.1002/adma.201204075 http://doi.org/10.1002/adma.201204075 .

Luo, C.; Kyaw, A. K. K.; Perez, L. A.; Patel, S.; Wang, M.; Grimm, B.; Bazan, G. C.; Kramer, E. J.; Heeger, A. J . General strategy for self-assembly of highly oriented nanocrystalline semiconducting polymers with high mobility . Nano Lett. , 2014 , 14 2764 - 2771 . DOI: 10.1021/nl500758w http://doi.org/10.1021/nl500758w .

Bucella, S. G.; Luzio, A.; Gann, E.; Thomsen, L.; McNeill, C. R.; Pace, G.; Perinot, A.; Chen, Z.; Facchetti, A.; Caironi, M . Macroscopic and high-throughput printing of aligned nanostructured polymer semiconductors for MHz large-area electronics . Nat. Commun. , 2015 , 6 8394 DOI: 10.1038/ncomms9394 http://doi.org/10.1038/ncomms9394 .

Giri, G.; Verploegen, E.; Mannsfeld, S. C. B.; Atahan-Evrenk, S.; Kim, D. H.; Lee, S. Y.; Becerril, H. A.; Aspuru-Guzik, A.; Toney, M. F.; Bao, Z . Tuning charge transport in solution-sheared organic semiconductors using lattice strain . Nature , 2011 , 480 504 - 508 . DOI: 10.1038/nature10683 http://doi.org/10.1038/nature10683 .

Zhang, L.; Liu, H.; Zhao, Y.; Sun, X.; Wen, Y.; Guo, Y.; Gao, X.; Di, C.; Yu, G.; Liu, Y . Inkjet printing high-resolution, large-area graphene patterns by coffee-ring lithography . Adv. Mater. , 2012 , 24 436 - 440 . DOI: 10.1002/adma.201103620 http://doi.org/10.1002/adma.201103620 .

Jiang, Y.; Chen, J.; Sun, Y.; Li, Q.; Cai, Z.; Li, J.; Guo, Y.; Hu, W.; Liu, Y . Fast deposition of aligning edge-on polymers for high-mobility ambipolar transistors . Adv. Mater. , 2019 , 31 1805761 DOI: 10.1002/adma.201805761 http://doi.org/10.1002/adma.201805761 .

Chen, L.; Chi, S.; Zhao, K.; Liu, J.; Yu, X.; Han, Y . Aligned films of the DPP-based conjugated polymer by solvent vapor enhanced drop casting . Polymer , 2016 , 104 123 - 129 . DOI: 10.1016/j.polymer.2016.10.005 http://doi.org/10.1016/j.polymer.2016.10.005 .

Zhao, Z.; Liu, H.; Zhao, Y.; Cheng, C.; Zhao, J.; Tang, Q.; Zhang, G.; Liu, Y . Anisotropic charge-carrier transport in high-mobility donor–acceptor conjugated polymer semiconductor films . Chem. Asian J. , 2016 , 11 2725 - 2729 . DOI: 10.1002/asia.201600082 http://doi.org/10.1002/asia.201600082 .

E. H. Gerhard Klink, A. Drost, D. Hemmetzberger, K. Bock, Conference Polytronic 2005 , Oct. 23–26 , Wroclaw, Poland , 2005 .

Kang, B.; Lee, W. H.; Cho, K . Recent advances in organic transistor printing processes . ACS Appl. Mater. Interfaces , 2013 , 5 2302 - 2315 . DOI: 10.1021/am302796z http://doi.org/10.1021/am302796z .

Stucchi, E.; Dell’Erba, G.; Colpani, P.; Kim, Y. H.; Caironi, M . Low-voltage, printed, all-polymer integrated circuits employing a low-leakage and high-yield polymer dielectric . Adv. Electr. Mater. , 2018 , 4 1800340 DOI: 10.1002/aelm.201800340 http://doi.org/10.1002/aelm.201800340 .

Yuvaraja, S.; Nawaz, A.; Liu, Q.; Dubal, D.; Surya, S. G.; Salama, K. N.; Sonar, P. . Organic field-effect transistor-based flexible sensors . Chem. Soc. Rev. , 2020 , 49 3423 - 3460 . DOI: 10.1039/C9CS00811J http://doi.org/10.1039/C9CS00811J .

Liu, K.; Ouyang, B.; Guo, X.; Guo, Y.; Liu, Y . Advances in flexible organic field-effect transistors and their applications for flexible electronics . npj Flex Electr. , 2022 , 6 1 DOI: 10.1038/s41528-022-00133-3 http://doi.org/10.1038/s41528-022-00133-3 .

Lee, Y. H.; Jang, M.; Lee, M. Y.; Kweon, O. Y.; Oh, J. H . Flexible field-effect transistor-type sensors based on conjugated molecules . Chem , 2017 , 3 724 - 763 . DOI: 10.1016/j.chempr.2017.10.005 http://doi.org/10.1016/j.chempr.2017.10.005 .

Ma, L.; Yi, Z.; Wang, S.; Liu, Y.; Zhan, X . Highly sensitive thin film phototransistors based on a copolymer of benzodithiophene and diketopyrrolopyrrole . J. Mater. Chem. C , 2015 , 3 1942 - 1948 . DOI: 10.1039/C4TC02462A http://doi.org/10.1039/C4TC02462A .

Qin, M. C.; Li, Q.-Y.; Zhang, F.; Liu, K.; Liu, Y. W.; Zhu, M. L.; Zhao, Z. Y.; Pan, Z. C.; Bian, Y. S.; Guo, Y. L.; Liu, Y. Q . High performance near-infrared organic photodetectors based on narrow-bandgap diketopyrrolopyrrole-based polymer . Acta Polymerica Sinica (in Chinese) , 2022 , 53 405 - 413 .

Gu, P . Hao.; Du, S.; Xie, C. Y.; Cai, B. M.; Zhang, S.; Shi, Y. X. 74-2: The excellent mechanical properties of novel polymer film and it’s application in the foldable AMOLED displays . SID Sympos. Digest of Technical Papers , 2019 , 50 1056 - 1059 . DOI: 10.1002/sdtp.13109 http://doi.org/10.1002/sdtp.13109 .

Liu, Y.; Zhao, Z.; Zhu, M.; Huang, X.; Wei, X.; Chen, H.; Chen, J.; Guo, Y.; Liu, Y . Realizing diketopyrrolopyrrole polymer-based uniform large-area transistors for active circuit via protonic acid mediated molecular self-assembly . Adv. Electr. Mater. , 2022 , 8 2100881 DOI: 10.1002/aelm.202100881 http://doi.org/10.1002/aelm.202100881 .

Views

930

Downloads

CSCD

Alert me when the article has been cited

Submit

Tools

Publicity Resources

Synergistic Effects of Solvent Vapor Assisted Spin-coating and Thermal Annealing on Enhancing the Carrier Mobility of Poly(3-hexylthiophene) Field-effect Transistors

Dimethylacetamide-promoted Direct Arylation Polycondensation of 6,6′-Dibromo-7,7′-diazaisoindigo and (E)-1,2-bis(3,4-difluorothien-2-yl)ethene toward High Molecular Weight n-Type Conjugated Polymers

Synthesis of Conjugated Polymers Containing Diketopyrrolopyrrole (DPP) Building Block and the Photophysical Study

Improvements of Hydrophobicity and Toughness of Epoxy Coatings Modified with Hydroxyl-terminated Fluororubber

Special Topic: Chirality in Polymers

Related Author

Xiao-Lan Qiao

Jie Yang

Lian-He Han

Ji-Dong Zhang

Mei-Fang Zhu

Kai Guo

Yu Jiang

Ying Sui

Related Institution

State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Donghua University

State Key Laboratory of Polymer Physics and Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences

School of Materials Science and Engineering, Tianjin University

Tianjin Key Laboratory of Molecular Optoelectronic Science, Tianjin University, and Collaborative Innovation Center of Chemical Science and Engineering (Tianjin)

Department of Polymer Science and Engineering, College of Chemistry, Chemical Engineering and Materials Science, Soochow University

⁰