Diketopyrrolopyrrole-based Conjugated Polymers as Representative Semiconductors for High-Performance Organic Thin-Film Transistors and Circuits

Kai-Qing Liu; Yuan-He Gu; Zheng-Ran Yi; Yun-Qi Liu

doi:10.1007/s10118-023-2943-1

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Diketopyrrolopyrrole-based Conjugated Polymers as Representative Semiconductors for High-Performance Organic Thin-Film Transistors and Circuits

REVIEW | Updated：2023-04-21

- Diketopyrrolopyrrole-based Conjugated Polymers as Representative Semiconductors for High-Performance Organic Thin-Film Transistors and Circuits
- Chinese Journal of Polymer Science Vol. 41, Issue 5, Pages: 671-682(2023)
- Affiliations：
  
  a.Zhuhai Fudan Innovation Institution, Zhuhai 518057, China
  b.Department of Environmental Science and Engineering, Faculty of Innovation Engineering, Macau University of Science and Technology, Macau 999078, China
  c.Key Laboratory of Organic Solids, Beijing National Laboratory for Molecular Sciences, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China
- Author bio：
  
  yzr@whu.edu.cn(Z.R.Y.)
  liuyq@iccas.ac.cn(Y.Q.L.)
- Funds：
- DOI：10.1007/s10118-023-2943-1
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Kai-Qing Liu, Yuan-He Gu, Zheng-Ran Yi, et al. Diketopyrrolopyrrole-based Conjugated Polymers as Representative Semiconductors for High-Performance Organic Thin-Film Transistors and Circuits. [J]. Chinese Journal of Polymer Science 41(5):671-682(2023)
DOI：

Kai-Qing Liu, Yuan-He Gu, Zheng-Ran Yi, et al. Diketopyrrolopyrrole-based Conjugated Polymers as Representative Semiconductors for High-Performance Organic Thin-Film Transistors and Circuits. [J]. Chinese Journal of Polymer Science 41(5):671-682(2023) DOI： 10.1007/s10118-023-2943-1.

摘要

The review summarizes the progress in molecular design, synthesis and solution-processing of DPP-based conjugated polymers for OTFT devices and circuits. The important roles of design strategies, synthesis methods and processing techniques are highlighted and discussed.

Abstract

Since the first report of diketopyrrolopyrrole (DPP)-based conjugated polymers for organic thin-film transistors (OTFTs), these polymers have attracted great attention as representative semiconductors in high-performance OTFTs. Through unremitting efforts in molecular-structure regulation and device optimization, significant mobilities exceeding 10 cm,2,·V,–1,·s,–1,have been achieved in OTFTs, greatly promoting the applied development of organic circuits. In this review, we summarize our progress in molecular design, synthesis and solution-processing of DPP-based conjugated polymers for OTFT devices and circuits, focusing on the roles of design strategies, synthesis methods and processing techniques. Furthermore, the remaining issues and future outlook in the field are briefly discussed.

关键词

Keywords

DiketopyrrolopyrrolePolymer semiconductorsOrganic thin-film transistorOrganic circuits

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State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Donghua University

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Department of Polymer Science and Engineering, College of Chemistry, Chemical Engineering and Materials Science, Soochow University

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